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Microwave assisted construction of Ag-AgBr reduced TiO2 nano-tube arrays photoelectrode and its enhanced visible light photocatalytic performance for degradation of 4-chlorphenol
Cheng, Qingfeng; Deng, Xiaoyong; Zhang, Huixuan; Guo, Ruonan; Cui, Yuqi; Ma, Qiuling; Zhang, Xinyi; Cheng, Xiuwen; Xie, Mingzheng; Li, Bo
第一作者Cheng, Qingfeng
2018-03-20
发表期刊SEPARATION AND PURIFICATION TECHNOLOGY
ISSN1383-5866
卷号193页码:255-263
摘要There is an increasingly significant issue on decomposition of contaminants in modem chemical industry and environmental protection. Hence, in the study, to improve the catalytic of semiconductor materials, the silver silver bromide nanoparticles decorated reduced TiO2 nano-tube arrays photoelectrode (Ag-AgBr/r-TiO2 NTAs), which exhibits better photocatalytic (PC) performance in the wide range of solar spectra, was successfully fabricated by anodization process, followed by microwave reduction strategy. The partly reduced AgBr nano particles are decorated and both Ti3+ and states are simultaneously introduced in the TiO2 NTAs photo electrode inducing the formation of impurity energy level to form Ag-AgBr/r-TiO2 NTAs photoelectrode. Moreover, PC activity of Ag-AgBr/r-TiO2 NTAs photoelelctrode was measured by degradation of 4-chlorphenol (4-CP). Results suggest that Ag-AgBr/r-TiO2 NTAs photoelectrode exhibits higher PC activity (99.9%) than that of other samples within 120 min illumination. The well combination of surface plasmons Ag-AgBr nanoparticles and r-TiO2 NTAs was responsible for the enhancing of PC, and the recombination of photo-generated electrons and holes can simultaneously be inhibited. Thus, Ag-AgBr nanoparticles and Ti3+ exert huge influence on the PC and photoelectrochemical properties of Ag-AgBr/r-TiO2 NTAs photoelectrode.
DOI10.1016/j.seppur.2017.10.068
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文献类型期刊论文
条目标识符http://ir.isl.ac.cn/handle/363002/34435
专题盐湖资源综合利用工程技术中心
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Cheng, Qingfeng,Deng, Xiaoyong,Zhang, Huixuan,et al. Microwave assisted construction of Ag-AgBr reduced TiO2 nano-tube arrays photoelectrode and its enhanced visible light photocatalytic performance for degradation of 4-chlorphenol[J]. SEPARATION AND PURIFICATION TECHNOLOGY,2018,193:255-263.
APA Cheng, Qingfeng.,Deng, Xiaoyong.,Zhang, Huixuan.,Guo, Ruonan.,Cui, Yuqi.,...&Li, Bo.(2018).Microwave assisted construction of Ag-AgBr reduced TiO2 nano-tube arrays photoelectrode and its enhanced visible light photocatalytic performance for degradation of 4-chlorphenol.SEPARATION AND PURIFICATION TECHNOLOGY,193,255-263.
MLA Cheng, Qingfeng,et al."Microwave assisted construction of Ag-AgBr reduced TiO2 nano-tube arrays photoelectrode and its enhanced visible light photocatalytic performance for degradation of 4-chlorphenol".SEPARATION AND PURIFICATION TECHNOLOGY 193(2018):255-263.
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