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A novel strategy to fabricate plasmonic Ag_AgBr nano-particle and its enhanced visible photocatalytic performance and mechanism for degradation of acetaminophen
Ma, Qiuling; Zhang, Huixuan; Guo, Ruonan; Cui, Yuqi; Deng, Xiaoyong; Cheng, Xiuwen; Xie, Mingzheng; Cheng, Qingfeng; Li, Bo
第一作者Ma, Qiuling
2017-11
发表期刊JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS
ISSN1876-1070
卷号80页码:176-183
摘要In the present work, plasmonic AgiAgBr nano-Particle was fabricated by solution reduction strategy. Meanwhile, physicochemical properties of the resulting samples were investigated by series of techniques. Results showed that Ag/AgBr nano-particle exhibited intense light absorbance in the whole visible region, high photoinduced charge separation efficiency and visible light driven PC performance. Furthermore, the enhanced visible light PC mechanism was proposed and confirmed. Besides, the PC degradation pathways of acetaminophen were elucidated based on the UPLC-MS/MS measurement. Results indicated that five degradation intermediates were detected, consequently two tentative pathways for PC degradation of acetaminophen were proposed, for example hydroxylation addition to parent compound and C N cleavage of side chain from the acetaminophen attacked by photoinduced holes. This study provides a facile and feasible strategy to fabricate high-efficient visible light response of nano-materials which can be applied in the fields of waste water treatment. (C) 2017 Taiwan Institute of Chemical Engineers. Published by Elsevier B.V. All rights reserved.
DOI10.1016/j.jtice.2017.06.033
引用统计
文献类型期刊论文
条目标识符http://ir.isl.ac.cn/handle/363002/34565
专题盐湖资源综合利用工程技术中心
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Ma, Qiuling,Zhang, Huixuan,Guo, Ruonan,et al. A novel strategy to fabricate plasmonic Ag_AgBr nano-particle and its enhanced visible photocatalytic performance and mechanism for degradation of acetaminophen[J]. JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS,2017,80:176-183.
APA Ma, Qiuling.,Zhang, Huixuan.,Guo, Ruonan.,Cui, Yuqi.,Deng, Xiaoyong.,...&Li, Bo.(2017).A novel strategy to fabricate plasmonic Ag_AgBr nano-particle and its enhanced visible photocatalytic performance and mechanism for degradation of acetaminophen.JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS,80,176-183.
MLA Ma, Qiuling,et al."A novel strategy to fabricate plasmonic Ag_AgBr nano-particle and its enhanced visible photocatalytic performance and mechanism for degradation of acetaminophen".JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS 80(2017):176-183.
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