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A solid-state electrochemical sensing platform based on a supramolecular hydrogel
Fu, Li; Wang, Aiwu; Lyu, Fucong; Lai, Guosong; Yu, Jinhong; Lin, Cheng-Te; Liu, Zhong; Yu, Aimin; Su, Weitao
2018-06-01
发表期刊SENSORS AND ACTUATORS B-CHEMICAL
ISSN0925-4005
卷号262页码:326-333
关键词Chitosan Hydrogel Electrochemical Sensing Platform Depolymerization Hydroxyl Radical
摘要Supramolecular hydrogels formed from the biopolymer chitosan and zinc ions were used as disposable electrochemical sensing platforms for the determination of hydroxyl radicals and hydrogen peroxide for the first time. The enclosed chitosan hydrogel served as the electrolyte for the system. In the presence of hydroxyl radicals or hydrogen peroxide, the chitosan hydrogel underwent depolymerization, resulting in the release of zinc ions from complexes formed with the hydrogel. The changes in the current from the zinc ions were then monitored and used as a signal for determining the concentration of analyte. The proposed chitosan hydrogel sensing platform exhibited a comparable detection performance with wide linear ranges and low detection limits for the two analytes. The linear detection range could be further manipulated by varying the depolymerization time. Due to the low cost and simplicity of the preparation process, this enzyme- and DNA-free sensing platform possesses great potential for application in disposable point-of-care devices and in-field testing. Additionally, the application of the proposed chitosan hydrogel to antioxidant screening could be further explored. (C) 2018 Published by Elsevier B.V.
DOI10.1016/j.snb.2018.02.029
语种英语
引用统计
文献类型期刊论文
条目标识符http://ir.isl.ac.cn/handle/363002/6443
专题青海盐湖研究所知识仓储
盐湖资源与化学实验室
推荐引用方式
GB/T 7714
Fu, Li,Wang, Aiwu,Lyu, Fucong,et al. A solid-state electrochemical sensing platform based on a supramolecular hydrogel[J]. SENSORS AND ACTUATORS B-CHEMICAL,2018,262:326-333.
APA Fu, Li.,Wang, Aiwu.,Lyu, Fucong.,Lai, Guosong.,Yu, Jinhong.,...&Su, Weitao.(2018).A solid-state electrochemical sensing platform based on a supramolecular hydrogel.SENSORS AND ACTUATORS B-CHEMICAL,262,326-333.
MLA Fu, Li,et al."A solid-state electrochemical sensing platform based on a supramolecular hydrogel".SENSORS AND ACTUATORS B-CHEMICAL 262(2018):326-333.
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