Synthesis of ZnFe2O4_B,N-codoped biochar via microwave-assisted pyrolysis for enhancing adsorption-photocatalytic elimination of tetracycline hydrochloride | |
Peng, Hao; Li, Yanxiang; Wen, Jing![]() | |
第一作者 | Peng, Hao |
2021-11-15 | |
发表期刊 | INDUSTRIAL CROPS AND PRODUCTS
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ISSN | 0926-6690 |
卷号 | 172 |
摘要 | B, N-codoped biochar was modified by ZnFe2O4 (ZnFe/BN-biochar) via the one-pot microwave-assisted pyrolysis for enhancing the adsorption-photocatalytic elimination of tetracycline hydrochloride (TCH). The addition of ZnFe2O4 could enhance the adsorption and photocatalytic capacity of B,N-codoped carbon under solar light irradiation. Among these composites, the optimal 3-ZnFe/3b-BN-biochar could remove 98.19 % of 150 mg L-1 TCH solution within 120 min, and its adsorption capacity estimated by Langmuir was 244.34 mg g(-1) for TCH removal. However, the removal efficiency of TCH over 3-ZnFe/3b-BN-biochar decreased to 89.45 % after seven cycles. The photocatalytic and adsorption kinetics of biochar-based composites for TCH removal were well descried with Langmuir-Hinshelwood and second-order models, respectively. In addition, Langmuir well fitted with the adsorption isotherms of biochar-based composites. The adsorption process of TCH over 3-ZnFe/3b-BN-biochar was a spontaneous and physisorption process. Hence, 3-ZnFe/3b-BN-biochar was a promising material for the adsorption and photocatalytic elimination of pollutants in wastewater. |
DOI | 10.1016/j.indcrop.2021.114066 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.isl.ac.cn/handle/363002/34382 |
专题 | 盐湖资源与化学实验室 |
推荐引用方式 GB/T 7714 | Peng, Hao,Li, Yanxiang,Wen, Jing,et al. Synthesis of ZnFe2O4_B,N-codoped biochar via microwave-assisted pyrolysis for enhancing adsorption-photocatalytic elimination of tetracycline hydrochloride[J]. INDUSTRIAL CROPS AND PRODUCTS,2021,172. |
APA | Peng, Hao,Li, Yanxiang,Wen, Jing,&Zheng, Xiaogang.(2021).Synthesis of ZnFe2O4_B,N-codoped biochar via microwave-assisted pyrolysis for enhancing adsorption-photocatalytic elimination of tetracycline hydrochloride.INDUSTRIAL CROPS AND PRODUCTS,172. |
MLA | Peng, Hao,et al."Synthesis of ZnFe2O4_B,N-codoped biochar via microwave-assisted pyrolysis for enhancing adsorption-photocatalytic elimination of tetracycline hydrochloride".INDUSTRIAL CROPS AND PRODUCTS 172(2021). |
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